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MS Excel Spreadsheet - 10.1 KB - SHA-256: 3fe34398a94338c247459461879624fcfeb90df747203b16e645d6ac74d6ade2
Table A2. Calculated speciation of 226Ra (CRa = 2·10-8 mol L-1) and saturation indices (SI) for Ra-phases in synthetic Opalinus Clay pore water after Pearson (1998).
MS Excel Spreadsheet - 11.2 KB - SHA-256: 01f2a3b2a3d71435aa89cb61e48b33b7d76370ce3c3c45903fef266bb61fb062
Table A5. Experimental data of 226Ra sorption kinetics on sandy Opalinus Clay at pH 7.6 and I = 0.39 mol·L-1 (cf. Fig. 9).
MS Excel Spreadsheet - 10.3 KB - SHA-256: 68ea1268ce1e355179728d875aa303a5a1316a96154d05cd21dd166fa15014f8
Table A6 . Experimental data of 226Ra sorption on sandy Opalinus Clay as a function of the S/L ratio at pH 7.6 and I = 0.39 mol·L-1 (cf. Fig. 12).
MS Excel Spreadsheet - 10.7 KB - SHA-256: b269d5b09fae86ae8bb6cb432ec76b92e1ccb8c955fe4fa185d0106f17958476
Table A3. Mineralogical composition (in wt.%) of rock samples from the lower sandy facies of the Opalinus Clay at Mont Terri taken from drill cores BDB-1 (Lerouge et al., 2015; Waber and Rufer, 2017) and BWS-H (Houben et al., 2014).
MS Excel Spreadsheet - 10.3 KB - SHA-256: 87256c87ca8ef13bd5996f8c3b1dcd6b27a3a728766bbf2e022f68ba0ddfff01
Table A1. Chemical composition (mol·L-1) of the different pore-waters in equilibrium with each clay sample and used in the sorption experiments in comparison to the synthetic Opalinus Clay pore water after Pearson (1998).
MS Word - 21.0 KB - SHA-256: 743b8a35fa0eccd586baabe0538b3916c658ea3027a60d42db0afb64222956eb
Figure A2. Predicted mole fractions of BaSO4 and SrSO4 in (Sr,Ba)SO4 celestite solid solution, whose fraction in the system is fixed at 0.4 wt. % of the total solid.
MS Word - 330.5 KB - SHA-256: c5d4953e1df4cf6111f43daa20b3527a97c4b2d67c57f584365f342ef0aabdb4
Figure A1. (Left) Representation of the mineralogical composition of rock samples from the lower sandy Opalinus Clay facies from drill core BAD-1 in a ternary diagram QFM (quartz, feldspar, and mica) – clay minerals – carbonates; (Right) lithotype classification of organic mudsto...
MS Excel Spreadsheet - 9.5 KB - SHA-256: df39db1e70cb4d95f48de2e93ca0d699f53a84b4125dfddcc9efd8a1d574bb58
Table A4. Result of EDS spot analyses of (Ba, Sr)-sulphate from the lower sandy Opalinus Clay facies (cf. Fig. 8).
MS Excel Spreadsheet - 139.9 KB - SHA-256: abe6e302465a0947e8f5c04684fe13c900bfeb3e76bcc551b4898d1274f9329a
Comma Separated Values - 18.5 KB - SHA-256: 14fe768d8541056c2b1e5cb2519179698c2b42bbb1e80786a2a387fb20042e1d
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